Nuclear Safety

Jacopo Buongiorno

Associa t e Pr of essor of Nuc l ear Science and Engineering

22.06 : Engineering of Nuclear Systems

Hazard

A very large inventory of radioactive fission products

(>GCi/t U ) ,

s ome w ith long half - life (>years)

R a d i o n u c l i d e c o n t e n t o f r e p r e s e n t a t i v e L W R s p e n t f u e l a t d i s c h a r g e a n d 1 8 0 d a y s o f r e p r e s e n t a t i v e L M F B R f u e l a t d i s c h a r g e a n d 3 0 d a y s

A c t i v i t y , C i / t m e t a l

L W R f u e l L M F B R f u e l

N u c l i d e

H a l f - l i f e

T 1 / 2

R a d i a t i o n s

D i s c h a r g e

1 8 0 d

D i s c h a r g e

3 0 d

1 2 . 3 y

5 . 7 4 4 x 1 0 2

5 . 5 8 7 x 1 0 2

1 . 6 4 8 x 1 0 3

1 . 6 4 0 x 1 0 3

1 0 . 7 3 y

1 . 1 0 8 x 1 0 4

1 . 0 7 4 x 1 0 4

1 . 4 7 3 x 1 0 4

1 . 4 6 6 x 1 0 4

5 0 . 5 d

1 . 0 5 8 x 1 0 6

9 . 6 0 3 x 1 0 4

1 . 3 3 3 x 1 0 6

8 . 9 3 9 x 1 0 5

2 0 . 9 y

8 . 4 2 5 x 1 0 4

8 . 3 2 3 x 1 0 4

9 . 5 9 1 x 1 0 4

9 . 5 7 2 x 1 0 4

6 4 . 0 h

8 . 8 5 0 x 1 0 4

8 . 3 2 5 x 1 0 4

1 . 2 1 4 x 1 0 5

9 . 5 7 2 x 1 0 4

5 9 . 0 d

1 . 2 6 3 x 1 0 6

1 . 5 2 5 x 1 0 5

1 . 7 9 4 x 1 0 6

1 . 2 6 9 x 1 0 6

6 4 . 0 d

1 . 6 3 7 x 1 0 6

2 . 4 3 7 x 1 0 5

3 . 2 1 5 x 1 0 6

2 . 3 4 0 x 1 0 6

3 . 5 0 d

1 . 5 5 7 x 1 0 6

4 . 6 8 9 x 1 0 5

3 . 1 4 9 x 1 0 6

2 . 9 5 4 x 1 0 6

6 6 . 0 h

1 . 8 7 5 x 1 0 6

3 . 7 8 0 x 1 0 - 1 4

4 . 0 4 0 x 1 0 6

2 . 1 0 8 x 1 0 3

6 . 0 h

1 . 6 1 8 x 1 0 6

3 . 5 8 9 x 1 0 - 1 4

3 . 4 8 7 x 1 0 6

2 . 0 0 2 x 1 0 3

2 . 1 x 1 0 5 y

1 . 4 3 5 x 1 0 1

1 . 4 4 2 x 1 0 1

3 . 2 7 8 x 1 0 1

3 . 2 9 3 x 1 0 1

Image by MIT OpenCourseWare.

3 H

8 5 K r

8 9 S r

9 0 S r

9 0 Y

9 1 Y

9 5 Z r

9 5 N b

9 9 M o

9 9 m T c 9 9 T c

Overarching O bjective of Nuclear Safety

Protect staff, public and environment

Preven t uncontrolle d releas e o f radioactivit y fro m p lant

I mp l emen t a ti on

- H eat removal

- D efense-in-depth:

Physical barriers

Design, construction and operation

Heat Removal

98% of all fission products are retained in the fuel pellet unless t he fuel melts

It is important to keep the fuel “cool” under all modes of normal o p eration:

1) Power mode (steady-state): fission energy generates steam which releases energy in turbine and condenser

2) Shutdown mode (turbine not available): decay heat generates steam, which is dumped directly into con d enser (PWR an d BWR) or a t mosp h ere ( on l y PWR)

3) Refueling mode: fuel is kept under water and decay heat is removed by residual heat removal system (RHRS)

Defense - in - Depth (physical barriers)

There exist multiple physical barriers between the source of radioactivity (the fission products) and the environment/public. The most important barriers are:

1 ) Fuel p ellet: it retains most solid fission p roducts.

2) Cladding: it retains all fission products (gaseous included).

3) Reactor c oolant system: robust h igh - pressure system of pipes + vessel. Most fission products are soluble in coolant and/or deposit on cold surfaces of pipes.

4) Containment: seal tight system is the ultimate barrier to radioactivity release, even if all previous barriers have failed .

D e f e n se -in-D ep th ( desi g n , construction and o p eration )

The concept of defense-of-depth extends to nuclear plant design, construction and operation.

Emphasis is on prevention, protection and mitigation .

1) Prevention. Minimize causes of failures/accidents before they occur:

- D esign reactor with inherent safety features (e.g. negative mo d era t o r , coo l an t an d f ue l reac ti v it y coe ff i c i en t s ) an d margins to failure (e.g. MDNBR>1.3)

- Use o f c hemically compatible materials ( e.g. no graphite and water in core)

- Q uality assurance in component manufacturing and construction (“N-stamp”)

- T horough training of operators + conservative operation

Defense - in - Depth (design ,

c onstruction and operation) (2)

2) Protection. Reactor protection system:

- M onitors plant conditions (e.g. measures temperature, pressure, flo w , powe r , radiation levels)

- R ecognizes precursors to transients/accidents

- A ctuates scram and safet y s y stems

3) Mitigation. When accidents do occu r , mitigate consequences using:

- E ngineered safety systems

- E mergency plan/evacuation

Desi g n-Basis Accident Classification

Undercooling: decrease in secondary-side heat removal (e . g . loss of condenser cooling water)

Overcooling: increase in secondary-side heat

removal ( e . g . loss of feedwater heating)

Overfilling: increase in reactor coolant inventory

(e . g . m ismatch between feedwater and steam flow

in BWR)

Loss o f flow: decrease i n c ore flow r ate ( e.g. trip of reactor pumps)

Loss of coolant: decrease of reactor coolant inventory (e.g. break of primary system pipe)

Desi g n-Basis Accident Classification ( 2 )

Reactivity insertion: uncontrolled insertion of positive

reactivity (e . g . r od drop in BWR)

Anticipated Transients Without Scram (ATWS): a relativel y fre q uent abnormal event ( transient ) with simultaneous failure to scram (e.g. loss of feedwater without scram)

Spent fuel accidents: occurring while handling and storing spent fuel assemblies (e.g. drop a fuel assembly , or critical configuration in fuel storage pool)

External events: an event initiating outside the plant

(e . g .

earthquake ,

hurricane ,

airplane crash)

En g in ee r ed Sa f e t y Sys t e m s

Functions

Shut - down reactor (i . e . stop the chain reaction) and keep reactor subcritical

Remove decay heat

R elieve pressure

M aintain ( or re p lenish ) reactor coolant inventor y

Requirements

Redundancy

D i v e r s i t y

Physical s eparation

En g in ee r ed Sa f e t y Sys t e m s ( 2 )

Shut-down reactor:

1) Scram c ontrol r ods (fast a cting: <2 sec)

2) Stand-by boron injection (slower acting, never used)

Remove decay heat:

1) Residual Heat Removal System (RHRS) in PWRs and BWRs, o r Isolation Condenser (IC) only in BWRs

BWR exam p le

Courtesy of GE Hitachi Nuclear Systems. Used with permission.

En g in ee r ed Sa f e t y Sys t e m s (3)

Remove decay heat (cont.):

2 ) Emer g enc y Feedwate r S y stem ( EFWS ) in PWRs and BWRs

- = M a i n f e e d w a t e r s y s t e m

S G = S t e a m G e n e r a t o r

C S T = C o n d e n s a t e s t o r a g e t a n k

Image by MIT OpenCourseWare.

Note redundanc y , diversity and physical separation

M. Gavrilas et al., Safety features of Operating LWRs of Western Design, CRC Press, 1995

En g in ee r ed Sa f e t y Sys t e m s ( 4 )

Relieve pressure

1) BWR: Safety/Relief V a lves (S R V s) located on main steam lines

2) PWR: Safety V a lves and Power Operated Relief Va l ve ( P O R V) l ocated o n top o f p r essu riz er

S R Vs and PO R V dischar g e steam into water pools located inside the containment

Courtesy of GE Hitachi Nuclear Systems. Used with permission.

Maintain (or replenish) reactor coolant inventory

The E mer gency Core Cooling S ystem ( ECCS) c omprises:

High Pressure Coolant Injection (HPCI) kicks in at high P (e.g. <12.5 MPa in PWR)

A ccumu l a t ors ki c k i n a t i n t erme di a t e P ( e. g . < 4 - 5 MP a i n PWR)

Low Pressure Coolant Injection (LPCI) kicks in at low P (i.e. 0.1 MPa)

Figures showing the BWR Emergency Feedwater System (EFWS) and the PWR accumulator.

En g ineered Safet y S y stems ( 5 )

Note:

- A ll ECCS water is highly borated

- HPCI an d LPCI are t yp i ca ll y ac ti ve (b ase d on pumps powere d b y emer gency diesel generators) in some advanced L W Rs they can be passive (no pumps or diesels needed)

Image by MIT OpenCourseWare.

M. Gavr ilas et al., Safety featur es of Oper ating LW Rs of W e ster n Design, CRC Pr ess, 1995

Large - Break LOCA

Double-guillotine rupture of the lar g est pipe in primary system, i . e ., cold leg between pump and vessel .

Never happened. It is the worst design-basis accident for L W Rs.

Historicall y ,

Sequence:

treated as a bounding event .

1) System depressurizes ( blowdown ) and empties very quickly (<20 sec). Can do nothing about this because it s so rapid. Note that the r eactor becomes s ubcritical even if CRs are not inserted, why?

At this p oint the core is uncovered. If nothin g is done , it would melt, why?

15

Large - Break LOCA (2)

2) ECCS (LPCI) kicks i n t o r e fill the v essel a nd r e flood the core. Refill and reflood take a few minutes.

If ECCS fails durin g refill and reflood , one has a severe accident (partial or complete melting of the core). However , ECCS is

designed to be redundant and diverse.

Some advanced L W Rs have passive ECCS. All existing L W Rs in U.S. have active ECCS, i.e., refill and reflood is done with pumps.

Note that ECCS water is heavily borated. Why?

16

Large - Break LOCA (3)

Legal limits for LB-LOCAs

Pl an t mus t sa ti s f y th e f o ll ow i ng requ i remen t s d ur i ng a LB - LOCA :

No fuel melting

Peak Cladding T e mperature (PCT) below 1204 C (2200 F), to prevent runaway Zr-steam reaction

Zr+2 H 2 O 2 ZrO 2 +2 H 2 +6500 kJ/kg Zr

Max oxidation of cladding <17% of original thickness, to prevent cladding failure

Less than 1% cladding oxidation average, to prevent excessive hydrogen production

No fuel “ballooning”, to maintain coolable geometry in core

Large - Break LOCA (4)

Analysis of LOCAs:

Entire d ivisions at vendors t o d o L B - LOCA analysis , importance.

given its

Sophisticated codes s uch a s R ELAP ( US) , T RAC ( US) ,

C A THARE (Europe), MARS (Korea) used for analysis. They all have the same architecture.

System is sectionalized and time-dependent conservation equations (mass, momentum, ener gy) are applied to each section.

Solving e quations numerically the P , T , f low a nd other u seful

parameters can be calculated as a function of time in each section. Neutronic behavior (not very important in LB-LOCAs) is s i mu l ate d w i t h s i mp l e ki net i c mo d e l .

18

Lar g e-Break LOCA ( 5 )

Example of RELAP nodalization for LB-LOCA analysis

28 6

28 0

27 0

1 7 0

17 2 17 4

27 2 27 4

27 8

27 1

15 8

18 6

18 0

17 8

17 1

28 2

01

18 2

20 4

10 8

18 4

28 4

1 7 6

2 76

15 0

20 6 20 2

15 2

20 0

31 0

35 6

03

35 5

35 0

31 1

10 6

10 0

10 4

10 2

11 0

20 9 21 0 21 2 21 4

20 8

BR E A K

01

30 0

30 5

31 5

08

04

32 8

34 5

34 0

32 0

33 3

06

01

33 0

32 5

32 2

33 5

01

01

30 1

30 6

31 6

08

19 4

11 8

11 6

SI

11 4

11 3

11 2

19 2

A C C

B r oke n Loo p

32 3

I n t a ct Lo op (L u m pe d)

3 intact loops are lumped into one with functioning LPCI train

Lar g e-Break LOCA ( 6 )

Most limiti ng constraint is PCT<1200 C

PCT has two peaks. Blowdown peak (coolant stagnates after break + ener gy redistributes ) and reflood p eak ( refill + q uenchin g) .

Depending on operating conditions and ECCS design, either blowdown peak or reflood peak is most limiti ng.

Large - Break LOCA (7)

Conservatism in LB-LOCA analysis (mandatory for licensing analyses)

1) Stored ener gy (important in blowdown): i nitial f uel T determined using h eat transfer and thermal conductivit y correlations yielding highest T

2) Decay heat vs time (important in reflood): use ANS standard +20%

3) Dischar g e rate through break is calculated using the Moody s model (overestimates dischar g e rate)

4) No return to nucleate boiling after DNB has been exceeded during blowdown. Return to nucleate boiling is allowed during reflood

5) Conservative film boiling correlations to be used

6) Failure of one ECCS train must be assumed (single failure rule)

PCT predicted with these assumptions is usually much higher than realit y , as demonstrated in LOFT e x periment at INL in the 80s .

The Containment

It encapsulates the “nuclear island” + performs three functions

1. Public and Environment Protection

Retention of radioactivity

Retention o f missiles

2. Protection of Plant Systems from

Natural elements (flood and storms)

Human actions (crashes and ex plosions, acts of sabotage)

Fires

3 . Structural Support o f S ystems

Routine service loads

Seismic loads

Internal loads during accidents

The Containment ( 2 )

- It is a reinforced-concrete building to perform functions 2 (protection from external events) and 3 (structural support)

- It has a steel liner to perform function 1 (retention of radioactivity)

S e i s m i c r e i n f o r c e m e n t

h 2

h

6

S h e a r t i e

h 5

h 3 h 4

h 1

A x i a l r e i n f o r c e m e n t H o o p r e i n f o r c e m e n t

Image by MIT OpenCourseWare.

Sy st em 80+™ Tech Papers, ANS M t g., AB B - C E , 1992.

The Containment ( 3 )

The most serious design-basis challenge to the containment is pressurization following a LB-LOCA

Energy “sources”:

- Primary system inventory

- Decay heat

- Chemical reactions (Zr-H 2 O, H 2 detonation)

- Stored energy in hot structures

Image by MIT OpenCourseWare.

The Containment ( 4 )

Two basic types of containment:

1) Pressur e containment . Desi g ned lar g e enou g h to accommodate all mass/energy without exceeding pressure limit during initial spike

2) Pressure-suppressio n containment . To mitigate the initial pressure

spike , i t u ses:

- S uppression pools or

- I ce condensers

Long-term (beyond initial pressure spike) all containments need:

- S prays (keep pressure low + scrub containment atmosphere)

- H 2 /O 2 recom bi ners o r N 2 i nert i zat i on ( prevent H 2 d etonat i on )

- D edicated heat exchangers (keep containment cool)

- Venting t hrough filters m ade of gravel ,

sand ,

water ,

e tc .

(done in Sweden, France, Germany, not US)

The Containment (5)

Pressure containment Pressure suppression containment (large and dry) (ice condensers)

B& W , “Steam , Its Generation & Use,” 1972. Sequoyah nuclear power plant

© Babcock & Wilcox. All rights reserved. This content is excluded from our Creative Commons license. For more information, see http://ocw.mit.edu/fairuse .

© source unknown. All rights reserved. This content is excluded from our Creative Commons license. For more information, see http://ocw.mit.edu/fairuse .

The Containment (6)

Pressure suppression

Pressure suppression containment

containment

(“ doughnut” suppression pool)

(suppression pool)

Image by MIT OpenCourseWare.

A. V . Nero, Jr ., A Guidebook to Nuclear Reactors , 1979.

© University of CA press. All rights reserved. This content is excluded from our Creative Commons license. For more information, see http://ocw.mit.edu/fairuse .

Source: Nero, Anthony V. A Guidebook to Nuclear Reactors.

Berkeley, CA: University of CA Pr, 1979. ISBN: 9780520036611.

The C ontainment (7)

Typical design parameters for US containments

P l a n t / T y p e

D e s i g n P r e s s u r e ( k P a )

T o t a l C o n t a i n m e n t F r e e V o l u m e ( m 3 )

A l l o w a b l e L e a k R a t e ( v o l % / d a y )

C a p a b i l i t y P r e s s u r e ( k P a )

L i m e r i c k / B W R M a r k - I I

4 8 0

1 1 , 6 0 0

0 . 5

1 0 6 6

G r a n d G u l f / B W R M a r k - I I I

2 0 4

4 7 , 3 0 0

0 . 4

5 1 5

S e q u o y a h / P W R I c e C o n d e n s e r

1 8 4

3 4 , 0 0 0

0 . 2 5

4 4 6

P e a c h B o t t o m / B W R M a r k - I

5 2 8

8 , 0 0 0

0 . 5

9 0 8

Z i o n / P W R L a r g e D r y

4 2 5

7 3 , 6 0 0

0 . 1

1 0 2 4

S u r r y / P W R S u b a t m o s p h e r i c

4 1 1

5 1 , 0 0 0

0 . 1

9 2 1

Image by MIT OpenCourseWare.

Be y ond-Desi g n-Basis ( “Severe” ) Accidents

Cause of severe accidents is inadequate fuel cooling , resulting in fuel melting

Can occur only with simultaneous failure of engineered safety systems

Sequence:

- LB - LOCA with failure of ECCS

- Fuel cladding damage and ballooning

- Coolant flow restriction due to deformed c ladding

- Fuel damage and fission product release

Noble g ases + volatile fission p roducts ( I , Br , Cs , Rb , Te , Se , Sr , Ba )

Non-volatile fission products remain with the fuel

Be y ond-Desi g n-Basis ( “Severe” ) Accidents ( 2 )

Sequence (cont.):

- Fuel melts and relocates to bottom of reactor vessel

- Molten fuel breaches vessel

- Molten fuel spreads on containment floor and is cooled (solidified) by water below vessel

- Concrete floor decom p osition results in g eneration of lar g e amounts of CO 2 which further pressurizes the containment

- H 2 from cladding/water reaction further pressurizes the containment

- If pressure is very high, containment can develop cracks and some fission products will escape into atmosphere

P l u m e

C l o u d s h i n e

F r e s h p r o d u c e

I m m e d i a t e I n h a l a t i o n i n g e s t i o n

F r e s h m i l k

S h i n e f r o m g r o u n d c o n t a m i n a t i o n ( g r o u n d s h i n e )

S k i n c o n t a m i n a t i o n

Be y ond-Desi g n-Basis ( “Severe” ) Accidents ( 3 )

Sequence (cont.):

- Fission products form a plume (cloud-shine) and can be transported to ground by settling and rain-out (ground-shine)

- Population is irradiated

Rai n

Pl u m e

S

Ho t Spo t

Image by MIT OpenCourseWare.

Em e r ge n cy Pl a n / Ev acua ti o n

Last resort. In case of severe accidents, if significant radioactivity release from the plant is expected, population within 10 miles

radiation exposure.

Seabrook Station

Qua ntifi ca ti o n o f N uc l ea r Ri s k

Risk (= frequency of an event its consequences) can be quantified through the use of Probabilistic Risk Assessment (PRA)

- A complex event (e.g. a nuclear accident) is broken into a sequence of individual events (e.g. failure of a safety pump, failure of a valve, containment bypass, etc), each with a given probability to occu r

- T he probability of the sequence is calculated using the formal rules of probabilities (essentially AND/OR logic operators)

- T he consequences of the event (e.g. human fatalities due to release of a certain amount of radioactivity) are calculated and risk curves (frequency vs consequences) can be constructed to compare the risk from various events, or even var i ous tec h no l og i es.

PRA was pioneered by the nuclear industr y , but its use is now wides p read , e. g . aviation and s p ace industr y, chemical industr y , economics, etc.

All about PRA in 22.38

Quantification of Nuclear Risk ( 2 )

A v e r a g e L o s s i n L i f e E x p e c t a n c y D u e t o V a r i o u s C a u s e s

From W A SH-1400, 1975

These numbers include the risk from severe accidents!

C a u s e

B e i n g u n m a r r i e d - m a l e C i g a r e t t e s m o k i n g - m a l e H e a r t d i s e a s e

B e i n g u n m a r r i e d - f e m a l e B e i n g 3 0 % o v e r w e i g h t B e i n g a c o a l m i n e r C a n c e r

C i g a r e t t e s m o k i n g - f e m a l e

L e s s t h a n e i g h t h - g r a d e e d u c a t i o n L i v i n g i n u n f a v o r a b l e s t a t e

S e r v i n g i n t h e U . S . a r m y i n V i e t n a m M o t o r v e h i c l e a c c i d e n t s

U s i n g a l c o h o l ( U . S . a v e r a g e ) B e i n g m u r d e r e d ( h o m i c i d e ) A c c i d e n t s f o r a v e r a g e j o b J o b w i t h r a d i a t i o n e x p o s u r e A c c i d e n t s f o r " s a f e s t " j o b

N a t u r a l b a c k g r o u n d r a d i a t i o n ( B E I R , 1 9 7 2 ) D r i n k i n g c o f f e e

O r a l c o n t r a c e p t i v e s

D r i n k i n g d i e t s o f t d r i n k s

R e a c t o r a c c i d e n t s ( K e n d a l l , 1 9 7 5 ) R e a c t o r a c c i d e n t s ( W a s h - 1 4 0 0 , 1 9 7 5 ) R a d i a t i o n f r o m n u c l e a r i n d u s t r y

P A P t e s t

S m o k e a l a r m i n h o m e A i r b a g s i n c a r

* * A s s u m e s t h a t a l l U . S . p o w e r i s n u c l e a r .

Image by MIT OpenCourseWare.

T i m e ( d a y s )

3 5 0 0

2 2 5 0

2 1 0 0

1 6 0 0

1 3 0 0

1 1 0 0

9 8 0

8 0 0

8 5 0

5 0 0

4 0 0

2 0 7

1 3 0

9 0

7 4

4 0

3 0

8

6

5

2

2 * *

0 . 0 2 * *

0 . 0 2 * *

- 4

- 1 0

- 5 0

Protect Public and Environment

Heat Removal

S teady-state

S hutdown

R efueling

Nuclear Safety

Defense in Depth

Ef fective Regulator (NRC) Peer Oversight (INPO)

Physical B arriers

Design ,

Construction and Operation

F uel pellet

C ladding

C oo l an t sys t em

C ontainment

P revention (inherently stable design, QA, operator training, conservative operation, etc.)

P ro t ec ti on ( reac t or pro t ec ti on sys t em )

M itigation:

- engineered safety systems

- emergency plan/evacuation

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22.06 Engineering of Nuclear Systems

Fall 20 10

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