Rad i at i o n Basi cs

C o okie pho to : Public domain .

22. S 902 D I Y G eiger C ount ers P rof . M ic hael S hort

Y ou hav e f our highly radioac t iv e c ook ies :

α β γ n

Y ou m us t :

P ut one in your pocket H old one in your hand E at one G ive one t o a “f riend”

O ld 2 2.01 Fi nal Exam Quest i o n

W hat do y ou do?

Co okie pho to : Pub lic domain . 2

M o t i vat i o n

I nt roduc e ioniz ing radiat ion bas ic s

E s t ablis h c om m on not at ion and t erm inology

U nders t and t y pes of radiat ion

I nt uit iv ely unders t and range of radiat ion

D eriv e and us e nuc lear reac t ion equat ions , half liv es of c om m on is ot opes

T y p es o f Io ni zi ng Rad i at i o n

A lpha ( α) Heliu m nucleu s +2

H eav y , c harged

± 1

B eta ( β ) A fr ee electr o n or positr on

Li ght, c harged

Gam m a ( γ) A nuclea r ph o ton ( l ight )

N o mas s , no c harge

Neutr on ( n ) A fr ee neutr on

H eav y , no c harge

Rang es o f Io ni zi ng Rad i at i o n

Graphic showing travel vs. blockage of alpha, beta, and gamma particles through 5 substances: paper, plastic, human hand, steel, and lead. Graphic showing travel vs. blockage of alpha, beta, and gamma particles through 5 substances: paper, plastic, human hand, steel, and lead. Graphic showing travel vs. blockage of alpha, beta, and gamma particles through 5 substances: paper, plastic, human hand, steel, and lead. Graphic showing travel vs. blockage of alpha, beta, and gamma particles through 5 substances: paper, plastic, human hand, steel, and lead.

P aper

Plastic

Steel

Lead

alpha beta beta

gamma

Image by MIT OpenCourseWare.

R elat i ve Ener g y Dep o si t i o n

Which do you think deposi ts the +2

m ost ener g y?

± 1

Wher e? ( Over what r ange ? )

Which type( s) is/ar e safer outside the body?

Which type( s) is/ar e safer inside the body?

Y ou hav e f our highly radioac t iv e c ook ies :

α β γ n

Y ou m us t :

P ut one in your pocket H old one in your hand E at one G ive one t o a “f riend”

O ld 2 2.01 Fi nal Exam Quest i o n

W hat do y ou do?

Co okie pho to : Public domain . 7

A tom s ar e deter m i n e d by the num be r of pr oton s

Exa m p le : He liu m A L W A YS h a s t wo p r o t o n s

T wo specia l types:

Io ns, Iso t o p es

Ion

S a m e # pr ot ons & neut r ons

Dif f er ent # elec t r ons ( c har ge)

Isotope

S a m e # pr ot ons

Ion A n at om wit h a c har ge ( dif f er ent # of pr ot ons & elec t r ons )

Is ot ope A n at om wit h a dif f er ent num ber of neut r ons ( m as s )

N ot a t ion

Dif f er ent # neut r ons ( m as s )

4 He

4 He

4 He +

3 He

Iso t o p i c No t at i o n

𝑍

± 𝑐

3 He

𝐴 𝑁𝑎𝑚 𝑒

A t om ic N um be r ( Z) T he num ber of pr ot ons in an at om

M ass Nu mb er ( A) T he t ot al num ber of nuc leons in an at om

N ot a t ion

Image No t a t i o n T empl at e

𝑈 = 𝑈

𝟗𝟗 𝟐𝟐𝟐𝟐 𝟎𝟎 𝟗𝟗 𝟐𝟐𝟐𝟐

𝟗𝟗𝟗𝟗

𝑈 = 𝑈

𝟗𝟗 𝟐𝟐𝟐𝟐 + 𝟒𝟒 𝟗𝟗 𝟐𝟐𝟐𝟐 + 𝟒𝟒

𝟗𝟗𝟗𝟗

𝟗𝟗𝟐𝟐

𝟔𝟔𝟎𝟎 𝐶𝑜 𝟎𝟎 = 𝟔𝟔𝟎𝟎 𝐶𝑜

No t at i o n Examp les

𝐶𝑠 =

1 𝟐𝟐𝟐𝟐 + 1

𝟐𝟐𝟐𝟐

𝟗𝟗

𝟒𝟒 𝐻 𝑒 + 𝟗𝟗 =

1 𝟐𝟐𝟐𝟐 𝐶𝑠 + 1

𝟒𝟒 𝐻 𝑒 + 𝟗𝟗 = 𝛂

St able Iso t o p es

S table isotopes do not under g o s p ont a neous

r adio a ctive decay

Which ar e stable? Consult the T abl e o f Nuclide s

Courtesy of K orea Atomic Energy Research Institute. Used with p ermiss ion.

S t a ble Is ot ope An is ot ope whic h does not under go s pont aneous , nat ur al r adioac t iv e dec ay

N ot a t ion

Look closer at one section

W hic h is ot opes of c hlor ine ar e s t able?

S a me n e u t r o n n u mb e r ( N)

St able Iso t o p es, At o mi c W ei g ht

http://atom.kaeri.re.kr/

S am e ato m i c n u mb e r ( Z )

St able Iso t o p es, At o mi c W ei g ht

http://atom.kaeri.re.kr/

Look closer at one section

W hic h is ot opes of c hlor ine ar e s t able? I n whic h per c ent ages ?

Look closer at one section

W hic h is ot opes of c hlor ine ar e s t able? I n whic h per c ent ages ?

𝑀𝑎 𝑠 𝑠 𝐶𝑙 =

Courtesy of Korea Atomic Energy Research Institute. Used with permission.

0. 7 5 7 7 3 4 . 98

0. 2 4 2 3 3 6 . 9 7

+

= 3 5 . 46 𝑎 𝑚𝑢

St able Iso t o p es, At o mi c W ei g ht

http://atom.kaeri.re.kr/

Li terat ure v al ue: 35 . 453 ± 0. 00 2 𝑎 𝑚𝑢

A t om ic W e ight T he av er age s t able elem ent is ot opic weight

At o mi c M ass Un i t ( amu ) Exa ct l y 1 12 t he weight of 12 𝐶

N ot a t ion

14

M o r e Feat ur es o f t he Nucli d e T able

http://atom.kaeri.re.kr/

E xcess M ass ( Δ) T he m as s of a nuc leus not ac c ount ed f or by t he weight of it s pr ot ons and neut r ons alone

N ot a t ion

Courtesy of K orea Atomic Energy Research Institute. Used with p ermiss ion.

E xcess m ass

Y ields ener get ic s and nuc lear r eac t ion inf or m at ion

S tability

Y ields half lif e and s pec if ic ac t iv it y inf or m at ion

P ar ent nuclide s

Y ields nuc lear r eac t ion m ec hanis m inf or m at ion

M o r e Feat ur es o f t he Nucli d e T able

http://atom.kaeri.re.kr/

E xcess m ass

Y ields ener get ic s and nuc lear r eac t ion inf or m at ion

S tability

Y ields half lif e and s pec if ic ac t iv it y inf or m at ion

M ode of decay

Y ields nuc lear r eac t ion

Hal f Lif e Th e ti m e i t t ak es 50% of an is ot ope t o dec ay

Decay E n erg y T he t ot al ener gy inv olv ed in t his r adioac t iv e dec ay

N ot a t ion

Courtesy of K ore a Atomic Energy Research Institute. U sed with p ermiss ion. m ec hanis m inf or m at ion

Next T hr ee T o p i cs

W rit ing nuc lear reac t ions

Q uant if y ing energet ic s of reac t ions

P redic t ing radiat ion t y pe and energy

Radio a ctive De ca y Natur al pr o cess

F ission S plitting atom s

T oday’ s focus

Nuclear R eact i o ns

T h e r m a l e n e r g y is co lle ct e d f r o m kin e t ic e n e r g y ( r e co il e n e r g y) o f f issio n p r o d u ct s

F usion Com bin i n g atom s

T h e r m a l e n e r g y is co lle ct e d f r o m m u lt ip le so u r ce s

Decay T he nat ur al pr oc es s of uns t able is ot ope c hange

Fis s ion T he pr oc es s of s plit t ing an is ot ope int o f is s ion f r agm ent s

Fus ion T he pr oc es s of c om bining t wo is ot opes int o a new one

N ot a t ion

18

Nuclear R eact i o n P r i nci p les

CONS E R V E ( alm ost) E V E R Y T HING

M as s ( num ber of nuc leons )

Char ge

E ner gy

NO T nec es s ar ily pr ot ons and neut r ons

E xam ple : T r itium decay 𝛼 + 2

𝟐𝟐 𝐻 𝟐𝟐 𝐻 𝑒 + ? ? ? 𝛽 ±

𝛾𝛾

Nuclear R eact i o n P r i nci p les ( β )

CONS E R V E ( alm ost) E V E R Y T HING

M as s ( num ber of nuc leons )

Char ge

E ner gy

NO T nec es s ar ily pr ot ons and neut r ons

E xam ple : T r itium decay

𝟐𝟐 𝐻 𝟐𝟐 𝐻 𝑒 + + 𝛽 + 𝐸 𝑟𝑥 𝑛

What is E rx n ? What else is m issing?

𝟐𝟐 𝐻 𝟐𝟐 𝐻 𝑒 + + 𝛽 + 𝐸 𝑟𝑥 𝑛

T otal E rx n : Look at dif fer en ce s in excess m ass

𝑀 𝑒𝑉

𝑄𝑄

= 𝑃 𝐷

Nuclear R eact i o n Ener g et i cs ( β )

T he Q value gives this am oun t

P ar ents ( P ) ar e all specie s on the left side

Daugh te r s ( D ) ar e all on the r ight side

𝟐𝟐 𝐻 𝟐𝟐 𝐻 𝑒 + +

~0

𝛽

+ 𝐸 𝑟𝑥 𝑛

Nuclear R eact i o n Ener g et i cs ( β )

http://atom.kaeri.re.kr/

𝑸

Courtesy of K orea Atomic Energy Research Institute. Used with p ermiss ion.

𝑀 𝑒 𝑉

= 𝑃 𝐷 = 1 𝟒𝟒 . 𝟗𝟗 𝟐𝟐𝟎𝟎 1 𝟒𝟒 . 𝟗𝟗 𝟐𝟐1 = 𝟎𝟎 . 𝟎𝟎 1𝟗𝟗 𝑀 𝑒 𝑉 22

𝟐𝟐 𝐻 𝟐𝟐 𝐻 𝑒 + + 𝛽 + 𝐸 𝑟𝑥 𝑛

T otal E rx n : Look at dif fer en ce s in excess m ass

𝑀 𝑒 𝑉

𝑸

= 𝑃 𝐷 = 1 𝟒𝟒 . 𝟗𝟗 𝟐𝟐𝟎𝟎 1 𝟒𝟒 . 𝟗𝟗 𝟐𝟐1 = 𝟎𝟎 . 𝟎𝟎 1𝟗𝟗 𝑀 𝑒 𝑉

Nuclear R eact i o n Ener g et i cs ( β )

Not all ener g y goes to the beta par ticle

A v er age bet a ener gy : 5. 7 ke V

S om e, not all, goes t o t he daught er nuc lide' s r ec oil

Wher e does the r est go?

3 𝐻 3 𝐻 𝑒 +

+ 𝛽 +

0 𝝂

+ 𝐸 𝑟𝑥 𝑛

Nuclear R eact i o n Ener g et i cs ( β )

0

An antine u tr in o car r ie s away the excess ener g y

Char g e le ss, essentia ll y m assless par ticle s

E xtr em ely har d to detect!

How did we know of their existence ? M issi n g ener g y in the r eaction ba l a n ce !

Neutr in o ( ν )

C hargel es s , n e a r ly m a ssle ss p a r t icle

A nti- neu tr in o ( ν )

A nti par ti c l e equi v al e nt of the neutr i no

C h e re n k o v ra d i a ti o n ri n g s p ro d u c e d b y

Courtesy of Kamioka Observatory, ICRR (Institute for Cosmic Ray Research), The University of Tokyo. Used with permission.

© Tomasz Barszczak. All rights reserved. This content is

Su p e r K am i o kan d e n e u tri n o d et ect o r , Jap an

25

excluded from our Creative Commons license. For more information, see http://ocw.mit.edu/help/faq-fair-use/ .

S om etim es beta decay leave s the nucleu s in an

excited state

T his ener g y can be lost thr ough gam m a em ission , br ing in g the nucle us to the gr oun d state

E xam ple : Cobalt- 60

D enotes excited

state

𝟔𝟔𝟎𝟎 𝐶𝑜

𝟔𝟔𝟎𝟎 𝑁𝑖 + + 𝛽 +

0 𝝂

Nuclear R eact i o n P r i nci p les ( γ )

0

𝟔𝟔𝟎𝟎 𝑁𝑖 +

𝟔𝟔𝟎𝟎 𝑁𝑖 + + γ

26

Nuclear R eact i o n P r i nci p les ( γ )

http://atom.kaeri.re.kr/

How to deter m i n e gam m a ener g y levels?

Use ener g y level diagr a m s

Nuclear R eact i o n P r i nci p les ( γ )

http://atom.kaeri.re.kr/

How c an t hi s be ?

I nt e r na l c onv e r si on c om pe t i ng pr oc e ss w i t h ga m m a e m i ss i on

Inter nal conver sio n ( IC)

Excit e d st a t e kicks o u t a n in n e r -sh e l l e le ct r o n

E xam ple : Cobalt- 6 0 m o st likely m echan ism

0

𝟔𝟔 𝟎𝟎 𝐶 𝑜 𝟔𝟔 𝟎𝟎 𝑁𝑖 + + 𝛽 +

0 𝝂 β

𝟔𝟔 𝟎𝟎 𝟗𝟗 . 𝟐𝟐1 𝑀 𝑒 𝑉 𝑁𝑖 + 𝟔𝟔 𝟎𝟎 𝟗𝟗 . 1 𝟔𝟔 𝑀 𝑒 𝑉 𝑁𝑖 +𝟗𝟗 + 𝑒 IC

Nuclear R eact i o n P r i nci p les ( γ )

𝟔𝟔 𝟎𝟎 𝟗𝟗 . 1 𝟔𝟔 𝑀 𝑒 𝑉 𝑁𝑖 +𝟗𝟗

𝟔𝟔 𝟎𝟎 1 . 𝟐𝟐𝟐𝟐 𝑀 𝑒 𝑉 𝑁𝑖 + 𝟗𝟗

𝟔𝟔 𝟎𝟎 1 . 𝟐𝟐𝟐𝟐 𝑀 𝑒 𝑉 𝑁𝑖 + 𝟗𝟗 + γ γ

𝟔𝟔 𝟎𝟎 𝑁𝑖 + 𝟗𝟗 + γ γ

29

Resul ting radiation spectrum can be complex

Example: Cesi um - 137

Nuclear R eacti on Princ iples ( γ )

Graph © Wiley-VCH, from J. Turner, Atoms, Radiation, and Radiation Protection (2007). All rights reserved. This content is excluded from our Creative Commons license. For more information, see http://ocw.mit.edu/help/faq-fair-use/ .

Courtesy of Korea Atomic Energy Research Institute. Used with permission.

30

Nuclear R eact i o n P r i nci p les ( γ )

http://atom.kaeri.re.kr/

Courtesy of K orea Atomic Energy Research Institute. Used with p ermiss ion. 31

Relative ly heavy isotope s can em it a heliu m nucleu s ( alpha par ticle)

E xam ple : A m er icium - 241

𝟗𝟗𝟒𝟒 1 𝐴 𝑚 𝟗𝟗 𝟐𝟐𝟐𝟐 𝑁𝑝 −𝟗𝟗 + α + 2

𝟗𝟗 𝟐𝟐𝟐𝟐 𝑁𝑝 𝟗𝟗

𝟗𝟗 𝟐𝟐𝟐𝟐 𝑁𝑝 𝟗𝟗 + γ

Nuclear R eact i o n P r i nci p les ( α )

32

Nuclear R eact i o n P r i nci p les ( α )

http:// en.wikipedia.org/wiki/Americium

Use s o f Am e r iciu m :

© MD111 on Flickr. License CC B Y -S A. This content i s excluded from our Creative

Commo ns license. For more information, see http://ocw.mit.edu/help/faq -f air - u se/ . 33

Nuclear R eact i o n P r i nci p les ( α )

http://atom.kaeri.re.kr/

Ho w' s t h i s d e ca y ch a in ?

Courtesy of Korea Atomic Energy Research Institute. Used with permission. 34

H alf L i fe

T im e it takes for half of an isotope to decay

T he decay constant r elates this to an expon e ntia l for m of the sam e r ule

1.0

0.693

T

A A 0

0.5

A = e - t

A 0

0.25

0.125

0

T

2T

3T

t

Image by MIT OpenCourseWare. 35

Define an activity in ter m s of decays per second

𝑑 𝑁

𝐴 =

𝑑 𝑡

= 𝜆𝑁 𝐴 = 𝐴 0 @ 𝑡 = 0

S olve the or din a r y dif fer en tia l equatio n :

𝑑𝑁

𝑡 = 0

𝑁 = −𝜆 𝑑 𝑡 ln 𝑁 = −𝜆 𝑡 + 𝑐 ln 𝑁 0 = 𝑐

ln 𝑁 = −𝜆 𝑡 + ln 𝑁 0

𝑁

𝑙𝑛

𝑁 0

= −𝜆 𝑡 𝑁 = 𝑁 0

𝑒 𝜆𝑡

H alf L i fe

λ descr ibe s how quickly the num b er of atom s N

chang e s by a factor of e

𝑑 𝑁

𝐴 = 𝑑 𝑡 = 𝜆𝑁 𝐴 = 𝐴 0 @ 𝑡 = 0

𝑁 = 𝑁 0

𝐴

𝜆

𝑒 −𝜆𝑡

= 𝐴 0

𝑒 𝜆𝑡

𝜆

Fi nd the hal f l i fe ( T ) :

𝑁

𝑁 0

= 1 = 𝑒 𝜆𝑇 ln 0. 5 = 𝜆𝑇 𝑇

2

0. 693

=

𝜆

H alf L i fe

Act i vi t y A m eas ur e of t he num ber of r adioac t iv e dec ay s per s ec ond Decay Co n st an t T he c ons t ant f or an ac t iv it y t o dec r eas e by a f ac t or of e H a lf Lif e T he t im e it t ak es a s am ple' s ac t iv it y t o dec r eas e by a f ac t or of 2

N ot a t ion

M easur i ng Act i vi t y

A ctivity is m easur e d in B ecquer e l s ( Bq )

1 𝐵𝑞 = 1 𝐷𝑖 𝑠𝑖 𝑛𝑡 𝑒 𝑔𝑟 𝑎𝑡 𝑖𝑜 𝑛 𝑝 𝑒𝑟 𝑠 𝑒𝑐 𝑜𝑛 𝑑

A m or e conveni e n t unit is the Cur ie ( Ci )

1 𝐶𝑖 = 3. 7 × 10 10 𝐵𝑞

Y ou will often see r educe d un i ts ( m Ci, µCi) o n r eal devices and sour ces

O n e Cu r ie is a l ot o f r a d ia t io n ! ! !

Becq u erel ( Bq ) T he f undam ent al unit of r adioac t iv it y , equal t o one dis int egr at ion per s ec ond

C ur ie ( C i) A m or e c onv enient ac t iv it y unit , 1 Ci = 3. 7 x 10 10 B q

N ot a t ion

© MD111 on Flickr. License CC B Y -SA . This content i s excluded from our Creative Commons license. For more information, see http://ocw.mit.edu/help/faq -fa ir -us e/ .

Label photo courtesy of Brooke Clarke. Used with permission. 39

T hi nki ng Ahead fo r t he L ab

How do you m easur e the activity of a sour ce?

How do you accoun t for older sour ces?

What else will m ake m easur i n g the activity of a sour ce dif ficult?

I n o t h e r wo r d s, wh a t a r e p o ssib le so u r ce s o f e r r o r and/or c onfus i on?

40

41

MIT OpenCourseWare http://ocw.mit.edu

22. S902 Do-It-Yourself (DIY) Geiger Counters

January IAP 2015

For information about citing these materials or our Terms of Use, visit: http://ocw.mit.edu/terms .